Notepad++ GUI and theme
Solution 1:
You can't change the application theme, however you can change toolbar for a start. Here's the toolbar with a set of tango icons;
Deviant Art Link (customisation tips in the comments)
There's a really interesting blog post (PaintBits - Improving Notepad++ into the perfect IDE), and a section on the NpWiki++ - Can I customise the toolbar? - both detailing how to customise Notepad++'s toolbar.
Theoretically you could re-purpose the following images to create your desired Chrome like toolbar;
WebAppers.com - Best Open Source Web Resources
As for tabs, their colour and font style can only be set;
Sadly there doesn't seem to an effort to bring all UI style configuration settings (toolbars, tabs, etc) under one setting (therefore no theme website you asked about). Perhaps suggest something on the Notepad++ Idea Tracker