Why are some of music files not being added to my iCloud Music Library?

Solution 1:

There's an option in the menus to force an update of the iCloud Music Library: File > Library > Update iCloud Music Library.

File > Library > Update iCloud Music Library

This caused a spinner to appear in the upper right-hand corner of iTunes and, once it disappeared, all my formerly-unavailable tracks were now available in my iCloud Music Library for streaming from my other devices.

Upper corner spinner

There was no need to log out and back in to my iTunes account.